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This is a 3:20 minutes long video, could you perhaps mention at which point the brush you’re referring to shows up?
I have seen this guy. He sells a pack of textured brushes that make the interesting effects when shading. They seem to be just textured brushes, nothing more. Here is a link to his pack just to show what they are, as we all know we can’t download them to Krita
Hello @fickledog and welcome to the community!
Do you mean these kinds of grainy brushes?
You can create them easily! I’ll take the b)Basic - 5 Size brush.
Go to the Brush Editor
And change the brush’s density. The lines I did in the first picture are 5%, 10%, 15%, 20%, 25%, and 30%, try different percentages and look for what you need. Then I changed the mask type from default to soft.
I went to General > Opacity (on the left side of the Editor) and checked Enable Pen Settings, then I went to General > Size and changed the curve:
Everything I wrote isn’t mandatory. Do what you want with your brushes, try different settings until you find your magical brush! 
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0:19 for example
Hello, @Katamaheen, this is exactly it! Thank you so much!
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You’re welcome! Glad I could help 
Another question. Do you know how could I make the grain more coarse? Basically increasing the individual particle size.
Maybe by giving a pattern to your brush? 
I don’t think you can increase the individual particle size, as it seems to be pixel-sized. So a small canvas will have “big” particles and a big canvas “small” ones.
If a pattern doesn’t help, then maybe try another brush, like that one:
I just took the original first brush and changed the brush tip in the Brush Editor; I clicked on predefined (between Auto and Text), and chose Sc_Scraches3, then in General, I checked Scatter and set the Strength to 30%. Again, try different brush tips (you can even do your own) and different settings until you find what you need!
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Thank you, I will try that!
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Or try amaking some brush with the spray engine.
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Check this thread - How About a Grain Brushes?
And this bundle seems to have some - Mojo Moo for comics
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Thank you!
For anyone reading, I’ve also found great success with spray brushes from Ramon!
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